Aerosol distribution in the northern Gulf of Guinea: local anthropogenic sources, long-range transport and the role of coastal shallow circulations

Autor: Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Alfons Schwarzenboeck, Julien Totems
Rok vydání: 2018
Popis: The complex vertical distribution of aerosols over coastal southern West Africa (SWA) is investigated using airborne observations and numerical simulations. Observations were gathered on 2 July 2016 offshore of Ghana and Togo, during the field phase of the Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa project. The aerosol loading in the lower troposphere includes emissions from coastal cities (Accra, Lomé, Cotonou and Lagos) as well as biomass burning aerosol and dust associated with long-range transport from Central Africa and the Sahara, respectively. Our results indicate that the aerosol distribution is impacted by subsidence associated with zonal and meridional regional scale overturning circulations associated with the land-sea surface temperature contrast and orography over Ghana and Togo. Numerical tracer release experiments highlight the dominance of aged emissions from Accra on the observed pollution plume loadings over the ocean. The contribution of aged emission from Lomé and Cotonou is also evident above the marine boundary layer. Lagos emissions do not play a role for the area west of Cotonou. The tracer plume does not extend very far south over the ocean (i.e. less than 100 km from Accra), mostly because emissions are transported northeastward near the surface over land and westward above the marine atmospheric boundary layer. The latter is possible due to interactions between the monsoon flow, complex terrain and land-sea breeze systems, which support the vertical mixing of the urban pollution. This work sheds light on the complex – and to date undocumented – mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated SWA region.
Databáze: OpenAIRE