Absence of superconductivity in topological metal ScInAu2

Autor: James Hamlin, J. M. DeStefano, J.B. Flahavan, T.A. Elmslie, Mark W. Meisel, G.P. Marciaga, U. S. Shah
Rok vydání: 2021
Předmět:
Zdroj: Physica C: Superconductivity and its Applications. 589:1353928
ISSN: 0921-4534
DOI: 10.1016/j.physc.2021.1353928
Popis: The Heusler compound S c I n A u 2 was previously reported to have a superconducting ground state with a critical temperature of 3.0K. Recent high throughput calculations have also predicted that the material harbors a topologically non-trivial band structure similar to that reported for β - P d B i 2 . In an effort to explore the interplay between the superconducting and topological properties properties, electrical resistance, magnetization, and x-ray diffraction measurements were performed on polycrystalline S c I n A u 2 . The data reveal that high-quality polycrystalline samples lack the superconducting transition present samples that have not been annealed. These results indicate the earlier reported superconductivity is non-intrinsic. Several compounds in the Au-In-Sc ternary phase space ( S c A u 2 , S c I n 3 , and S c 2 I n A u 2 ) were explored in an attempt to identify the secondary phase responsible for the non-intrinsic superconductivity. The results suggest that elemental In is responsible for the reported superconductivity in S c I n A u 2 .
Databáze: OpenAIRE