Analysis of cross-flow jet-type singlet oxygen generator

Autor: T. Fujioka, Daichi Sugimoto, K. Tei, G. Watanabe
Rok vydání: 2004
Předmět:
Zdroj: IEEE Journal of Quantum Electronics. 40:1030-1040
ISSN: 0018-9197
DOI: 10.1109/jqe.2004.831617
Popis: A cross-flow jet-type singlet oxygen generator has been developed, tested and analyzed in order to characterize the dependence of output performance on major input parameters. A thermal-balance model, which can predict O/sub 2/(/sup 1//spl Delta/) yield, gas temperature, and gas residence time, is proposed, and the resultant theoretical results are compared to the experimental data. Combined with computational fluid dynamics-based gas residence-time analysis, the model provides good agreement with the measured value of the O/sub 2/(/sup 1//spl Delta/) yield and the gas temperature. The surface chemistry model was applied to the measured Cl/sub 2/ utilization data, and was found to be inconsistent in the regime of high Cl/sub 2/ loading on the basic hydrogen peroxide jet, indicating that depletion of HO/sub 2//sup -/ is taking place.
Databáze: OpenAIRE