Graphitic carbon/carbon nitride hybrid as metal-free photocatalyst for enhancing hydrogen evolution
Autor: | Zheguan Lin, Zizhong Zhang, Xuxu Wang, Qi Liu, Yangen Zhou, Lu Chen, Yiqun Cao, Jinlin Long, Xiaohan An |
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Rok vydání: | 2017 |
Předmět: |
Diffuse reflectance infrared fourier transform
Process Chemistry and Technology Inorganic chemistry 02 engineering and technology 010402 general chemistry 021001 nanoscience & nanotechnology 01 natural sciences Catalysis 0104 chemical sciences Dielectric spectroscopy chemistry.chemical_compound symbols.namesake X-ray photoelectron spectroscopy Chemical engineering chemistry symbols Water splitting Beta carbon nitride 0210 nano-technology Raman spectroscopy Carbon nitride Hydrogen production |
Zdroj: | Applied Catalysis A: General. 546:30-35 |
ISSN: | 0926-860X |
DOI: | 10.1016/j.apcata.2017.07.046 |
Popis: | Graphitic carbon/carbon nitride hybrid was fabricated by a two-step procedure from the initially hydrothermal self-assembly of melamine and sucrose and then typical thermal condensation. The structure, composition, photoelectric and photocatalytic properties of the resulting sample was characterized in detail by X-ray diffraction, Fourier transform infrared spectra, Raman spectra, X-ray photoelectron spectroscopy, transmission electron microscopy, UV–vis diffuse reflectance spectroscopy, photoelectric current, electrochemical impedance spectroscopy and photocatalytic hydrogen production. The results revealed that the graphitic carbon/carbon nitride hybrid has conjugation effect between carbon nitride and graphitic carbon and thus leads to a better efficiency for water splitting than the pristine carbon nitride. |
Databáze: | OpenAIRE |
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