Novel graphitic-C3N4 nanosheets: enhanced visible light photocatalytic activity and photoelectrochemical detection of methylene blue dye

Autor: K. Y. Li, J. Luo, Z. L. Fang, S. Xiong
Rok vydání: 2017
Předmět:
Zdroj: Materials Technology. 32:391-398
ISSN: 1753-5557
1066-7857
DOI: 10.1080/10667857.2016.1262309
Popis: The graphitic–C3N4 nanosheets were synthesised via direct pyrolysis of melamine followed by a thermal exfoliation. The structure, morphology, optical, and electronic properties were explored by comprehensive characterisation methods and the photocatalytic activities of the graphitic-C3N4 nanosheets were evaluated by the degradation of Rhodamine B under visible light irradiation. Moreover, the graphitic-C3N4 nanosheets were used to determinate the concentration of methylene blue. The results showed that graphitic-C3N4 nanosheets have the same structural feature with that of the bulk-C3N4. The enhancing photocatalytic performance of the graphitic-C3N4 nanosheets results from the more absorption and active sites, the improving separation efficiency of photogenerated electron-hole pairs. Moreover, the photocurrent intensity decreased with the increasing of methylene blue concentration, which makes graphitic-C3N4 nanosheets a promising sensor material for estimating the concentration of methylene blue.
Databáze: OpenAIRE