Ultrafast Dynamics of Charge Density Waves in4Hb−TaSe2Probed by Femtosecond Electron Diffraction

Autor: Reinhard Birmurske, Heinrich Schwoerer, Jure Demsar, Maximilian Eichberger, Helmuth Berger, G. H. Kassier, N. Erasmus, Ilana Boshoff, K. Haupt
Rok vydání: 2012
Předmět:
Zdroj: Physical Review Letters. 109
ISSN: 1079-7114
0031-9007
DOI: 10.1103/physrevlett.109.167402
Popis: The dynamics of the photoinduced commensurate-to-incommensurate charge density wave (CDW) phase transition in 4H(b)-TaSe2 are investigated by femtosecond electron diffraction. In the perturbative regime, the CDW re-forms on a 150-ps time scale, which is two orders of magnitude slower than in other transition-metal dichalcogenides. We attribute this to a weak coupling between the CDW carrying T layers and thus demonstrate the importance of three-dimensionality for the existence of CDWs. With increasing optical excitation, the phase transition is achieved, showing a second-order character, in contrast to the first-order behavior in thermal equilibrium.
Databáze: OpenAIRE