Ultrafast Dynamics of Charge Density Waves in4Hb−TaSe2Probed by Femtosecond Electron Diffraction
Autor: | Reinhard Birmurske, Heinrich Schwoerer, Jure Demsar, Maximilian Eichberger, Helmuth Berger, G. H. Kassier, N. Erasmus, Ilana Boshoff, K. Haupt |
---|---|
Rok vydání: | 2012 |
Předmět: | |
Zdroj: | Physical Review Letters. 109 |
ISSN: | 1079-7114 0031-9007 |
DOI: | 10.1103/physrevlett.109.167402 |
Popis: | The dynamics of the photoinduced commensurate-to-incommensurate charge density wave (CDW) phase transition in 4H(b)-TaSe2 are investigated by femtosecond electron diffraction. In the perturbative regime, the CDW re-forms on a 150-ps time scale, which is two orders of magnitude slower than in other transition-metal dichalcogenides. We attribute this to a weak coupling between the CDW carrying T layers and thus demonstrate the importance of three-dimensionality for the existence of CDWs. With increasing optical excitation, the phase transition is achieved, showing a second-order character, in contrast to the first-order behavior in thermal equilibrium. |
Databáze: | OpenAIRE |
Externí odkaz: |