A comprehensive study of Interatomic Coulombic Decay in argon dimers: Extracting R-dependent absolute decay rates from the experiment
| Autor: | Přemysl Kolorenč, Joshua B. Williams, Markus Schöffler, Mo Zohrabi, Till Jahnke, N. Gehrken, A. Moradmand, Tsveta Miteva, Kirill Gokhberg, H. Sann, Allen Landers, Florian Trinter, Reinhard Dörner, Jonas Rist, I. Ben-Itzhak, M. Keiling, Th. Weber, Maksim Kunitski, Bishwanath Gaire, Ben Berry, Ali Belkacem |
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| Rok vydání: | 2017 |
| Předmět: |
Work (thermodynamics)
Decay scheme Argon Chemistry General Physics and Astronomy chemistry.chemical_element 02 engineering and technology Electron Radiation 021001 nanoscience & nanotechnology Kinetic energy 01 natural sciences Ion Interatomic Coulombic decay 0103 physical sciences Physics::Atomic and Molecular Clusters Physical and Theoretical Chemistry Atomic physics 010306 general physics 0210 nano-technology |
| Zdroj: | Chemical Physics. 482:185-191 |
| ISSN: | 0301-0104 |
| DOI: | 10.1016/j.chemphys.2016.09.024 |
| Popis: | In this work we present a comprehensive and detailed study of Interatomic Coulombic Decay (ICD) occurring after irradiating argon dimers with XUV-synchrotron radiation. A manifold of different decay channels is observed and the corresponding initial and final states are assigned. Additionally, the effect of nuclear dynamics on the ICD electron spectrum is examined for one specific decay channel. The internuclear distance-dependent width Γ ( R ) of the decay is obtained from the measured kinetic energy release distribution of the ions employing a classical nuclear dynamics model. |
| Databáze: | OpenAIRE |
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