Investigation of the natural radioactivity of volcanic rock samples using a low background gamma-ray spectrometer

Autor: Jurian Hoogewerff, Jan Hertogen, Va Sole, R. Wordel, D. Mouchel
Rok vydání: 1994
Předmět:
Zdroj: Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment. 339:322-328
ISSN: 0168-9002
DOI: 10.1016/0168-9002(94)91825-2
Popis: A low-level high-purity Ge detection system was used to investigate samples of volcanic rock from different locations. A lead shield surrounded the 100 cm 3 germanium crystal and reduced the background radioactivity by a factor of 100 within the energy interval 70 to 3000 keV; an integrated count rate of (0.498 ± 0.001) s −1 was achieved over this inverval, which was mainly attributable to the influence of cosmic rays. Although sample volumes up to 2 litres can be measured, the volcanic samples were held in cylindrical containers and varied in volume from 16 to 20 cm 3 . A powdered solid source was prepared of similar chemical composition to the samples, and spiked with suitable radionuclides to calibrate the detector system. The resulting efficiency calibration was compared with a Monte Carlo simulation of the detector efficiency for extended sources. Corrections were made for the given geometry, self-absorption and absorption in calculating the full energy-peak efficiency ( ϵ γ ). The concentrations of various radionuclides originating from the natural decay chains in the different samples were compared to a well known reference sample. A wide variation of the concentrations of the measured radionuclides and a breaking of secular equilibrium was observed.
Databáze: OpenAIRE