Design of UiO-66@BiOIO3 heterostructural composites with remarkable boosted photocatalytic activities in removing diverse industrial pollutants
| Autor: | Wang Xiaojian, Xue mei Qi, Shi ji Li, Qiang Wu, Ke xuan Li, Can Liu |
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| Rok vydání: | 2021 |
| Předmět: |
Pollutant
Materials science Composite number Light irradiation 02 engineering and technology General Chemistry 010402 general chemistry 021001 nanoscience & nanotechnology Condensed Matter Physics 01 natural sciences Decomposition 0104 chemical sciences law.invention chemistry.chemical_compound chemistry law Specific surface area Rhodamine B Photocatalysis General Materials Science Xenon arc lamp Composite material 0210 nano-technology |
| Zdroj: | Journal of Physics and Chemistry of Solids. 151:109903 |
| ISSN: | 0022-3697 |
| DOI: | 10.1016/j.jpcs.2020.109903 |
| Popis: | Novel UiO-66@BiOIO3-x composites have been successfully designed for the first time. The as-prepared UiO-66@BiOIO3-x composites exhibit superior photocatalytic activity for the decomposition of rhodamine B (RhB) and tetracycline (TC), compared with the corresponding BiOIO3. For UiO-66@BiOIO3-30 composite, approximately 93.2% of RhB and 88.4% of TC were decomposed under a 300 W xenon arc lamp light irradiation. Furthermore, the UiO-66@BiOIO3-50 composite presents outstanding oxidative removal activity for gaseous Hg0. The evident improvement of the photocatalytic property over the UiO-66@BiOIO3-x composites might be ascribed to the promoted separation efficiency of electron–hole pairs and the larger specific surface area. Finally, the electron-hole migration mechanism over UiO-66@ BiOIO3-50 composite is put forward in the light of trapping experiments. This research strategy will provide outstanding development in the application of photocatalysis. |
| Databáze: | OpenAIRE |
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