Direct observation of bulk second-harmonic generation inside a glass slide with tightly focused optical fields

Autor: Susobhan Das, Shima Fardad, Alessandro Salandrino, Xianghui Wang, Rongqing Hui
Rok vydání: 2016
Předmět:
Zdroj: Physical Review B. 93
ISSN: 2469-9969
2469-9950
DOI: 10.1103/physrevb.93.161109
Popis: Bulk second-harmonic generation (SHG) inside glass slides is directly detected unambiguously without interference from surface contributions. This is enabled by tightly focused and highly localized ultrashort laser pulses. The theoretical calculations based on vector diffraction theory and the phenomenological model of SHG inside centrosymmetric materials agree well with the measured far-field SHG radiation patterns for different polarization states of the fundamental beam. The results indicate that the observed bulk SHG is predominantly related to the bulk parameter ${\ensuremath{\delta}}^{\ensuremath{'}}$ and originates from the three-dimensional field gradient in the focal region.
Databáze: OpenAIRE