Theoretical study of the photocurrent in transition-metal dichalcogenide materials

Autor: Hyun C. Lee
Rok vydání: 2017
Předmět:
Zdroj: Physical Review B. 95
ISSN: 2469-9969
2469-9950
DOI: 10.1103/physrevb.95.245102
Popis: Motivated by photocurrent spectroscopy experiments with $\mathrm{Mo}{\mathrm{S}}_{2}$, the direct band-to-band transition contribution to the photocurrent of transition-metal dichalcogenides is computed starting from the microscopic Hamiltonian in the Keldysh-Schwinger formalism. It turns out that the band tilting induced by source to drain voltage is necessary for a nonvanishing photocurrent. The photon energy dependence of the normalized photocurrent is found to be consistent with experimental data. For circular polarization the helicity-dependent component of the photocurrent perpendicular to the band-tilting direction is predicted, which essentially originates from the valley Hall effect.
Databáze: OpenAIRE