Autor: |
Xuejie Guo, Jun Wang, Haocheng Yang |
Rok vydání: |
2022 |
Předmět: |
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Zdroj: |
Inorganic Chemistry Frontiers. 9:155-164 |
ISSN: |
2052-1553 |
DOI: |
10.1039/d1qi01203g |
Popis: |
Micro/mesoporous powder structures and biofouling of marine microorganisms directly limit the potential of zeolite frameworks in uranium recovery from seawater. Herein, an anti-biofouling zeolite framework-8/chitosan/melamine sponge adsorbent with a three-dimensional porous structure was prepared successfully using zinc ions and chitosan as adjuvants to promote the growth of zeolite framework-8 on the surface of melamine sponge. The mechanical and anti-biofouling properties of the sponge were determined by compression and algae tests. Relative to the zeolite framework-8 powders, the zeolite framework-8/chitosan/melamine sponge exhibited superior mechanical and anti-biofouling properties with 0.565 MPa of compressive stress and a 35% algae cell death rate. The adsorption capacities of the zeolite framework-8/chitosan/melamine sponge were 129.90 mg g−1 at pH 8.0 and 95.47 mg g−1 at the fifth adsorption–desorption cycle, which were higher than that of ZIF-8 powder (91.45 mg g−1). Furthermore, the excellent low-concentration U(VI) adsorption performance of zeolite framework-8/chitosan/melamine in natural seawater (Bohai) also confirmed its practical application potentiality. |
Databáze: |
OpenAIRE |
Externí odkaz: |
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