Hour-glass magnetic spectrum arising from a striped cluster spin-glass ground state in La1.75Sr0.25CoO4

Autor: Matthias Vojta, S. M. Gaw, Christopher D. Frost, D. Prabhakaran, Eric C. Andrade, D. T. Adroja, Andrew T. Boothroyd
Rok vydání: 2013
Předmět:
Zdroj: Physical Review B. 88
ISSN: 1550-235X
1098-0121
DOI: 10.1103/physrevb.88.165121
Popis: We report inelastic neutron scattering results that reveal an hour-glass magnetic excitation spectrum in La${}_{1.75}$Sr${}_{0.25}$CoO${}_{4}$. The magnetic spectrum is similar to that observed previously in La${}_{1.67}$Sr${}_{0.33}$CoO${}_{4}$, but the spectral features are broader. We show that the spectrum of La${}_{1.75}$Sr${}_{0.25}$CoO${}_{4}$ can be modelled by the spin dynamics of a system with a disordered cluster spin glass ground state. Bulk magnetization measurements are presented that support the proposed glassy ground state. The observations reiterate the importance of quasi-one-dimensional magnetic correlations and disorder for the hour-glass spectrum, and suggest that disordered spin and charge stripes exist at lower doping in La${}_{2\ensuremath{-}x}$Sr${}_{x}$CoO${}_{4}$ than previously thought.
Databáze: OpenAIRE