Strong coupling between Eu2+spins and Fe2As2layers in EuFe1.9Co0.1As2observed with NMR

Autor: Sergiy Katrych, S. Strässle, J. Karpinski, Alexander Shengelaya, Zurab Guguchia, F. Murányi, Alexander Maisuradze, Zbigniew Bukowski, Stephen Weyeneth, J. Roos, Hugo Keller
Rok vydání: 2011
Předmět:
Zdroj: Physical Review B. 83
ISSN: 1550-235X
1098-0121
DOI: 10.1103/physrevb.83.144516
Popis: A combination of x-ray diffraction, magnetization, and $^{75}\mathrm{As}$ nuclear magnetic resonance (NMR) experiments were performed on single-crystal EuFe${}_{1.9}$Co${}_{0.1}$As${}_{2}$. The strength of the hyperfine interaction between the $^{75}\mathrm{As}$ nuclei and the Eu${}^{2+}$ 4$f$ states suggests a strong coupling between the Eu${}^{2+}$ moments and the Fe${}_{1.9}$Co${}_{0.1}$As${}_{2}$ layers. Such a strong interlayer coupling may be due to an indirect exchange interaction between the localized Eu${}^{2+}$ 4$f$ moments, mediated by the Fe 3$d$ conduction electrons. Magnetic susceptibility as well as $^{75}\mathrm{As}$-NMR measurements reveal a decrease of the SDW transition temperature to ${T}_{\mathrm{SDW}}$ $=$ 120 K as a result of Co doping. A change of the slope in the temperature dependence of the NMR frequency of the $^{75}\mathrm{As}$ lower-satellite line was observed at 225 K. At the same temperature also a change of the satellite line shape was found. These changes of the NMR spectra may be caused by the formation of a nematic phase below 225 K in EuFe${}_{1.9}$Co${}_{0.1}$As${}_{2}$.
Databáze: OpenAIRE