Current progress of Pt-based ORR electrocatalysts for PEMFCs: An integrated view combining theory and experiment
Autor: | J.C. Ortiz-Herrera, H. Rojas-Chávez, Omar Solorza-Feria, E. López-Chávez, Pastor T. Matadamas-Ortiz, H. Cruz-Martínez, Dora I. Medina |
---|---|
Rok vydání: | 2021 |
Předmět: |
Materials science
Physics and Astronomy (miscellaneous) Fuel cells Oxygen reduction reaction General Materials Science Nanotechnology 02 engineering and technology 010402 general chemistry 021001 nanoscience & nanotechnology 0210 nano-technology 01 natural sciences 0104 chemical sciences Energy (miscellaneous) |
Zdroj: | Materials Today Physics. 19:100406 |
ISSN: | 2542-5293 |
DOI: | 10.1016/j.mtphys.2021.100406 |
Popis: | The sluggish kinetics of oxygen reduction reaction (ORR) affects the massive use of polymer exchange membrane fuel cells (PEMFCs). Therefore, the use of electrocatalysts is required to accelerate the ORR kinetics. Usually, Pt/C electrocatalysts are used for the ORR. Nevertheless, the principal disadvantages of using Pt are its high-cost, low availability, and limited stability. For these reasons, research of more stable and cost effective electrocatalysts with high electrocatalytic activity is important to achieve large-scale power generation. To date, there are significant advances and great opportunities for the design of novel electrocatalysts with high electrocatalytic activity and stability for the ORR through the connection of experimental and theoretical explorations. For these reasons, in this review, combined theoretical–experimental studies for the design of novel Pt-based metallic electrocatalysts for the ORR are revised and analyzed in detail. |
Databáze: | OpenAIRE |
Externí odkaz: |