Influence of the contact angle on two-phase flow in microreactors for nitrobenzene-hydrogen-stainless steel/carbon

Autor: Furkan Özkan, Kristin Hecht, Bettina Kraushaar-Czarnetzki, Klaus Schubert, Peter Pfeifer
Rok vydání: 2010
Předmět:
Zdroj: Surface and Interface Analysis. 42:1122-1127
ISSN: 1096-9918
0142-2421
DOI: 10.1002/sia.3386
Popis: The contact angle of a gas-liquid-solid system plays a significant role in predicting flow patterns in microchannels for multiphase flows. The contact angle, which is a result of surface forces, is strongly influenced by the channel material. In the present study, we describe contact angle measurements and simulations of flow in a microchannel for the multiphase system hydrogen and nitrobenzene. Contact angles for nitrobenzene-hydrogen-stainless steel and nitrobenzene-hydrogen-carbon systems were measured using the sessile drop method at various pressures. Simulation of the two-phase system was performed using ANSYS FLUENT. The static contact angle is used as a boundary condition. The results from simulation of flow for a wide range of contact angles and the measured contact angles are presented. Experimental observations and simulation results agree in that the contact angle must be smaller 90° to obtain small bubbles and to increase the gas-liquid interfacial surface area.
Databáze: OpenAIRE