Impacts of framework Al distribution and acidic properties of Cu-exchanged CHA-type zeolite on catalytic conversion of methane into methanol followed by lower hydrocarbons

Autor: Kengo Nakamura, Peipei Xiao, Ryota Osuga, Yong Wang, Shuhei Yasuda, Takeshi Matsumoto, Junko N. Kondo, Mizuho Yabushita, Atsushi Muramatsu, Hermann Gies, Toshiyuki Yokoi
Rok vydání: 2023
Předmět:
Zdroj: Catalysis Science & Technology. 13:2648-2651
ISSN: 2044-4761
2044-4753
DOI: 10.1039/d3cy00127j
Popis: This work highlighted the significance of the Al distribution in the CHA-type zeolite in the formation of active Cu species for the oxidative conversion of CH4; isolated Al atoms in the zeolite framework are found to be advantageous for producing CH3OH.
Databáze: OpenAIRE