Recent measurements of 36Cl in Yucca Mountain rock, soil and seepage

Autor: Klaus J. Stetzenbach, R. Howley, Y. Wei, James V. Cizdziel, Vernon F. Hodge, J. Cline, F. M. Phillips
Rok vydání: 2007
Předmět:
Zdroj: Journal of Radioanalytical and Nuclear Chemistry. 275:133-144
ISSN: 1588-2780
0236-5731
DOI: 10.1007/s10967-007-7002-9
Popis: Samples of rock, soil and seepage were collected from Yucca Mountain, USA, and analyzed for 36Cl/Cl ratios by accelerator mass spectrometry (AMS). Rock excavated from the Drill Hole Wash fault at repository horizon depths produced a ratio suggesting that small amounts of water with “bomb-pulse” 36Cl had percolated to that site over the past 50 years. Rock from four other sites within the exploratory studies facility did not yield bomb-pulse ratios. Ratios in the soil varied depending on depth and location, with some samples producing bomb-pulse signatures. Ratios for seep water were slightly elevated above the present cosmogenic background value. This paper also discusses results from a column study mimicking the passage of 36Cl through volcanic rock and from an experiment using bromide instead of chloride as a carrier in sample preparation for AMS.
Databáze: OpenAIRE