Pulse-stacked cavity ring-down spectroscopy
Autor: | Thomas G. Spence, H. A. Schwettman, Eric R. Crosson, P. Haar, Barbara A. Paldus, G. A. Marcus, Richard N. Zare |
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Rok vydání: | 1999 |
Předmět: | |
Zdroj: | Review of Scientific Instruments. 70:4-10 |
ISSN: | 1089-7623 0034-6748 |
Popis: | Pulse stacking, or synchronous pumping, is a novel approach that offers important advantages in cavity ring-down spectroscopy. Using an ultrashort pulse, high repetition rate laser source we have shown that it is possible to resonantly stack pulses in a high finesse cavity, significantly enhancing the decay wave forms obtained when the laser source is abruptly terminated. We have achieved signal-to-noise ratio improvements of several orders of magnitude compared to single pulse injection systems, demonstrating a sensitivity of 2×10−9 cm−1 at 5.38 μm. |
Databáze: | OpenAIRE |
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