The specifics of radiative annihilation of self-trapped excitons in a KI–Tl crystal under low-temperature deformation

Autor: Nurgul Zhanturina, A. A. Barmina, Z. Aimaganbetova, Sh. Zh. Sagymbaeva, L. Myasnikova, K. Sh. Shunkeyev, D. M. Sergeyev
Rok vydání: 2016
Předmět:
Zdroj: Low Temperature Physics. 42:580-583
ISSN: 1090-6517
1063-777X
DOI: 10.1063/1.4960008
Popis: The effect of low-temperature uniaxial deformation on the self-trapping-limited mean free path of excitons in a KI–Tl crystal was revealed from x-ray luminescence spectra. The analysis of the dependence of the intensity ratio of the Tl-center emission (2.85 eV) and the luminescence of self-trapped excitons (π-component; 3.3 eV) on the extent of low-temperature deformation showed that in the KI–Tl crystal (3 × 10−3 mol. %) the self-trapping-limited mean free path of excitons is comparable with the distance between Tl atoms (20–27)a under a deformation e = 2%. As the compression increases to e ≥ 2%–5%, the mean free path drops to (27-5.35)a. The results of modeling based on the continuum approximation showed that with increasing temperature and the degree of low-temperature deformation the height of the potential barrier for the exciton self-trapping drops, which is consistent with the reduction of the mean free path of excitons in the KI–Tl crystal.
Databáze: OpenAIRE