Thermal expansion of the spin-½ Heisenberg-chain compound Cu(C4H4N2)(NO3)2

Autor: M.D. Phillips, J. Rohrkamp, Thomas Lorenz, Mark M. Turnbull
Rok vydání: 2010
Předmět:
Zdroj: Journal of Physics: Conference Series. 200:012169
ISSN: 1742-6596
DOI: 10.1088/1742-6596/200/1/012169
Popis: Compounds containing magnetic subsystems representing simple model spin systems with weak magnetic coupling constants are ideal candidates to test theoretical predictions for the generic behavior close to quantum phase transitions. We present measurements of the thermal expansion and magnetostriction of the spin-½-chain compound copper pyrazine dinitrate Cu(C4H4N2)(NO3)2. Of particular interest is the low-temperature thermal expansion close to the saturation field Hc ≊ 13.9 T, which defines a quantum phase transition from the gapless Luttinger liquid state to the fully saturated state with a finite excitation gap. We observe a sign change of the thermal expansion for the different ground states, and at the quantum critical point Hc the low-temperature expansion approaches a divergence. Thus, our data agree very well with the expected quantum critical behaviour.
Databáze: OpenAIRE