Decoherence of ensembles of nitrogen-vacancy centers in diamond

Autor: Erik Bauch, Susanne Yelin, Matthew Turner, Swati Singh, Ronald L. Walsworth, Junghyun Lee, Jennifer Schloss, Connor A. Hart, Linh M. Pham, John Barry, Nir Bar-Gill
Rok vydání: 2020
Předmět:
Zdroj: Physical Review B. 102
ISSN: 2469-9969
2469-9950
DOI: 10.1103/physrevb.102.134210
Popis: We present a combined theoretical and experimental study of solid-state spin decoherence in an electronic spin bath, focusing specifically on ensembles of nitrogen-vacancy (NV) centers in diamond and the associated substitutional nitrogen spin bath. We perform measurements of NV spin free-induction decay (FID) times ${T}_{2}^{*}$ and spin-echo coherence times ${T}_{2}$ in 25 diamond samples with nitrogen concentrations [N] ranging from 0.01 to 300 ppm. We introduce a microscopic model and perform numerical simulations to quantitatively explain the degradation of both ${T}_{2}^{*}$ and ${T}_{2}$ over four orders of magnitude in [N]. Our analysis enables us to describe the NV ensemble spin coherence decay shapes as emerging consistently from the contribution of many individual NV centers.
Databáze: OpenAIRE