Infrared cavity ringdown and integrated cavity output spectroscopy for trace species monitoring

Autor: Janelle R. Anderson, Alfred Y. Cho, Federico Capasso, Anthony O'Keefe, L. B. Lapson, James J. Scherer, Joshua B. Paul, Claire F. Gmachl
Rok vydání: 2002
Předmět:
Zdroj: SPIE Proceedings.
ISSN: 0277-786X
DOI: 10.1117/12.455722
Popis: Although the ability of high finesse optical cavities to provide effective absorption path-lengths exceeding 10 km. has been known for quite some time, attempts to utilize this property for the purposes of high-resolution spectroscopy have often resulted in extremely complex experimental systems. Here, we demonstrate how off-axis optical paths through such cavities can be employed to produce relatively simple spectrometers capable of ultrasensitive absorption measurements. A proof-of-concept study using visible diode lasers has achieved a normalized absorption sensitivity of 1.8*10-10 cm-1Hz-1/2. Additionally, quantum cascade lasers have been employed to extend this method into the mid-infrared region, where sensitivities of 1.2*10-9 cm-1Hz-1/2 have been obtained.
Databáze: OpenAIRE