Transition of a small-bipolaron gas to a Fröhlich polaron in a deformable lattice

Autor: Mohd Nazlan Mohd Muhid, Gayan Prasad Hettiarachchi, Halimaton Hamdan
Rok vydání: 2018
Předmět:
Zdroj: Physical Review B. 97
ISSN: 2469-9969
2469-9950
DOI: 10.1103/physrevb.97.155142
Popis: The electronic properties of guest Cs atoms in a deformable lattice are investigated at various densities $n$. Low values of $n$ show optical absorptions of small bipolarons. At intermediate $n$ values, new bands appear in the midinfrared (MIR) and high-frequency regions, which coexist with the small bipolaron bands. With a further increase in $n$, the small bipolaron bands become less discernible and subsequently disappear, resulting in the appearance of a Drude component superimposed on a MIR sideband suggesting a phase transition to a polaronic metal. In this itinerant phase, an approximately twofold mass enhancement is observed. This continuous transition of a gas of small bipolarons to a polaronic metal characterized by a Fr\"ohlich polaron reveals an important part of the complex phase diagram of the metal-insulator transition in a deformable lattice.
Databáze: OpenAIRE