Direct evidence of uneven dxz and dyz orbital occupation in the superconducting state of iron pnictide

Autor: Zbigniew Bukowski, Marcin Matusiak, Michał Jurczyszyn, D. Rybicki, Marcin Sikora, Czesław Kapusta, Michal Babij, Joanna Stępień, Kamil Goc, Tomasz Strączek, Łukasz Gondek, M. Zając
Rok vydání: 2020
Předmět:
Zdroj: Physical Review B. 102
ISSN: 2469-9969
2469-9950
DOI: 10.1103/physrevb.102.195126
Popis: The origin of nematicity and its relation to superconductivity in iron pnictide high-temperature superconductors remains unclear. One of its possible sources is the uneven occupation of Fe ${d}_{xz}$ and ${d}_{yz}$ orbitals. Here, by using x-ray linear dichroism technique, we show that such an imbalance is present in $\mathrm{Eu}{({\mathrm{Fe}}_{1\ensuremath{-}x}{\mathrm{Co}}_{x})}_{2}{\mathrm{As}}_{2}$ single crystals deep in the tetragonal phase and also in the superconducting state, where we find that the ${d}_{xz}$ orbital has a higher occupation as indicated by an x-ray linear dichroism magnitude of 1.5%. Our result shows the importance of orbital polarization in the theoretical description of nematicity and superconductivity, particularly for determination of the superconducting gap symmetry, which is affected by orbital fluctuations.
Databáze: OpenAIRE