Versatility of iron-rich steel waste for the removal of high arsenic and sulfate concentrations in water
Autor: | Claudia L. Caldeira, Camila C. Amorim, Ariádna Andrade Saldanha da Silva, Sandrine F. Araujo, Virginia S.T. Ciminelli |
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Rok vydání: | 2018 |
Předmět: |
Basic oxygen steelmaking
Aqueous solution Environmental remediation Contact time Health Toxicology and Mutagenesis chemistry.chemical_element General Medicine 010501 environmental sciences Contamination Acid mine drainage 01 natural sciences Pollution chemistry.chemical_compound chemistry Environmental chemistry Environmental Chemistry Sulfate Arsenic 0105 earth and related environmental sciences |
Zdroj: | Environmental Science and Pollution Research. 26:4266-4276 |
ISSN: | 1614-7499 0944-1344 |
Popis: | The aim of this work is to evaluate the application of a steel waste, basic oxygen furnace sludge (BOFS), rich in iron, to treat water contaminated with elevated arsenic and sulfate concentrations. In the first step, three doses (10, 60, and 80 g L−1) of BOFS were tested to investigate the removal of As(III) and As(V) (67 mg L−1) and sulfate (3700 mg L−1) separately from an aqueous solution. In the second step, the efficacies of BOFS (10 g L−1) and commercial ZVI (5 g L−1) were compared to simultaneously remove arsenic and sulfate. The pH of the feed solution was adjusted to 2.5 and monitored during the experiment. The use of BOFS achieved arsenic removal up to 92% and sulfate removal of nearly 40% after 72 h of contact time. Use of BOFS also increased the solution pH to 12. Similar removal levels were achieved with both BOFS and ZVI. These results confirm the potential application of BOFS to remove high arsenic and sulfate concentrations from acidic solutions. The data obtained here should be used as a basis for further studies on the remediation of acid mine drainage with high concentrations of arsenic and sulfate using an abundant and low-cost steel waste. |
Databáze: | OpenAIRE |
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