High-temperature magnetic anomaly in the Kitaev hyperhoneycomb compound β-Li2IrO3

Autor: Ruiz, Alejandro, Nagarajan, Vikram, Vranas, Mayia, Lopez, Gilbert, McCandless, Gregory T, Kimchi, Itamar, Chan, Julia Y, Breznay, Nicholas P, Frañó, Alex, Frandsen, Benjamin A, Analytis, James G
Rok vydání: 2020
Předmět:
Zdroj: Physical Review B, vol 101, iss 7
Popis: We report the existence of a high-temperature magnetic anomaly in the three-dimensional Kitaev candidate material, β-Li2IrO3. Signatures of the anomaly appear in magnetization, heat capacity, and muon spin relaxation measurements. The onset coincides with a reordering of the principal axes of magnetization, which is thought to be connected to the onset of Kitaev-like correlations in the system. The anomaly also shows magnetic hysteresis with a spatially anisotropic magnitude that follows the spin-anisotropic exchange anisotropy of the underlying Kitaev Hamiltonian. We discuss possible scenarios for a bulk and impurity origin.
Databáze: OpenAIRE