Molecules in high-intensity laser fields

Autor: Nguyen-Dang, T.-T., Châteauneuf, F., Manoli, S.
Zdroj: Canadian Journal of Chemistry; June 1996, Vol. 74 Issue: 6 p1236-1247, 12p
Abstrakt: The separability of a dressed molecule, a composite molecule + quantized radiation field system, at high field intensities is examined. Various forms of the Hamiltonian describing the dressed molecule are reviewed and are used to assess the zeroth-order separability of the dressed system. A new high-order adiabatic separation between the strongly coupled quantized field and molecular subsystems is derived. Qualitative manifestations of laser-induced molecular structures are discussed within this high-order adiabatic representation. Keywords: dynamics, dressed molecule, intense laser field, adiabatic separation, laser-induced molecular structure.
Databáze: Supplemental Index