Excitation energy transfer and population dynamics in a quantum dot system induced by optical near-field interaction.

Autor: Sangu, S., Kobayashi, K., Shojiguchi, A., Kawazoe, T., Ohtsu, M.
Předmět:
Zdroj: Journal of Applied Physics; 3/1/2003, Vol. 93 Issue 5, p2937, 9p, 4 Diagrams, 5 Graphs
Abstrakt: Energy transfer and exciton population dynamics in a two-quantum dot system coupled with a phonon heat-bath system are examined using the density matrix formalism. In such a system, optical near-field interactions induce energy transfer between quantum dots, and exciton-phonon interactions guarantee the unidirectional excitation energy transfer. Our theoretical investigation shows that the population dynamics change drastically depending on the coupling strengths due to optical near-field interactions and exciton-phonon heat-bath interactions. The temperature effect promotes frequent energy back-transfer from the heat-bath to the quantum dot system. Applying our theoretical formulation, we numerically calculate the time evolution of populations, and estimate energy transfer time or state-filling time for a CuCl quantum dot system. The estimated time is suitable for the elements in our proposed optical nano-switch and nano-photonic devices. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index