Stationary and Time-Resolved Hot Luminescence of Self-Trapped Excitons in Rare Gas Crystals.

Autor: Selg, M., Hizhnyakov, V., Kink, R., Kink, M., Maksimov, J.
Zdroj: Journal of Low Temperature Physics; Feb2001, Vol. 122 Issue 3/4, p241-248, 8p
Abstrakt: Experimental (Xe, Kr) and theoretical (Xe) hot luminescence (HL) data are presented for the atomic cryocrystals Xe and Kr. The experimental spectra were registered under two-photon excimer laser (ArF and KrF) excitation. The theoretical treatment was based on a new nonperturbative quantum-mechanical relaxation theory, which predicts sharp acceleration of the decay rate around a characteristic “critical” vibrational level of a strong local mode. The time-resolved HL spectra were calculated for the quasi-molecules Xe*2 in solid Xe, taking account of all bound-bound and bound-free transitions in the centre. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index