Poly-3,4-ethylenedioxythiophene/Polystyrene Sulfonate/Dimethyl Sulfoxide-Based Conductive Fabrics for Wearable Electronics: Elucidating the Electrical Conductivity and Durability Properties through Controlled Doping and Washing Tests.

Autor: Aizamddin, Muhammad Faiz, Roslan, Nazreen Che, Ayub, Ayu Natasha, Sabere, Awis Sukarni Mohmad, Sofian, Zarif Mohamed, Chang, Yee Hui Robin, Mohd Ghazali, Mohd Ifwat, Sadasivuni, Kishor Kumar, Kasri, Mohamad Arif, Fakir, Muhamad Saipul, Mahat, Mohd Muzamir
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Zdroj: Journal of Polymer Materials; 2024, Vol. 41 Issue 4, p239-261, 23p
Abstrakt: Poly-3,4-ethylenedioxythiophene: polystyrene sulfonate (PEDOT/PSS) has revolutionized the field of smart textiles as an advanced conductive polymer, offering an unprecedented combination of high electrical conductivity, solution processability, and mechanical conformability. Despite extensive research in PEDOT/PSS-coated fabrics over the past decade, a critical challenge remains in finding the delicate balance between enhanced conductivity and washing durability required for real-world wearable applications. Hence, this study investigates the electrical conductivity and durability properties of PEDOT/PSS-based conductive fabrics for wearable electronics. By carefully controlling the doping concentration of dimethyl sulfoxide (DMSO), an optimal conductivity of 8.44 ± 0.21 × 10−3 S cm−1 was achieved at 5% DMSO. Durability was assessed through simulated washing tests of up to 30 cycles following standardized protocols. Although the fabric's conductivity decreased from 10−3 to 10−4 S cm−1 after the 5th wash, it stabilized at approximately ~5.67 ± 0.05 × 10−4 S cm−1 beyond the 30th cycle. These findings demonstrate the fabric's ability to retain its electrical properties under repeated washing, making it highly suitable for long-term use in wearable electronics. A range of characterization techniques—including attenuated total reflectance–Fourier transform infrared spectroscopy, Raman analysis, scanning electron microscopy–energy dispersive X-ray, X-ray diffraction, electrochemical impedance spectroscopy, and tensile testing—were employed to analyze the fabric's functional groups, morphology, crystallinity, conductivity, and mechanical properties. The results validate the robustness and applicability of PEDOT/PSS/DMSO fabrics for reliable performance in wearable electronic applications. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index
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