Rapid synthesis of ZnO nanoparticles via gliding arc discharge: unveiling the impact of discharge time on particle properties and photocatalytic performance.

Autor: Messai, Ridha, Ferhat, Mohammed Fouad, Serouti, Abdelghani, Nourelhouda, Bounedjar, Humayun, Muhammad, Allag, Nassiba, Zoukel, Abdelhalim, Ghezzar, Mouffok Redouane, Bououdina, Mohamed
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Zdroj: Environmental Science & Pollution Research; May2024, Vol. 31 Issue 23, p33885-33903, 19p
Abstrakt: Herein, we present a novel approach for the synthesis of ZnO nanoparticles (ZnO NPs) using a non-thermal plasma source generated by the gliding arc discharge-air system. The effect of discharge time on the physical and optical properties, as well as the photocatalytic performance of the as-fabricated ZnO NPs, was investigated. The characterization techniques revealed that the as-synthesized ZnO exhibit hexagonal Wurtzite structure, with a wide energy gap and peak intensities of UV–vis absorption with longer discharge times. A decrease in particle size from 29 to 25 nm was also observed with increasing discharge time, while all samples were thermally stable between 25 and 700 °C. The photocatalytic performance of the ZnO NPs was evaluated by degrading Congo Red (CR) dye with a concentration of 20 ppm under sunlight at a dose of 1 mg/mL. The as-synthesized ZnO NPs revealed exceptional photocatalytic performance by degrading ~ 97% of CR dye after irradiation for 150 min. This work presents an easy and simple method for synthesizing NPs in a short time and pave the way for other potential ideas on the application of plasma gliding arc discharge. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index