Stability and fragmentation processes of highly charged sodium clusters.

Autor: Ntamack, G. E., Chandezon, F., Manil, B., Lebius, H., Tomita, S., Guet, C., Njock, M. G. Kwato, Huber, B. A.
Předmět:
Zdroj: European Physical Journal D (EPJ D); Jun2003, Vol. 24 Issue 1-3, p153-156, 4p
Abstrakt: Highly charged sodium clusters produced in collisions between neutral clusters and multiply charged ions are formed within a large range of temperatures and fissilities, and identified by means of a high-resolution reflectron-type time-of-flight mass spectrometer ( m/δm ≈ 14000). The limit of stability of these charged clusters is experimentally investigated, and the time-of-flight spectra are compared with theoretical spectra based on Monte-Carlo simulations. The results indicate that the maximum fissility (X) of stable clusters is approaching the Rayleigh limit (X = 1) for larger clusters sizes. It is mainly limited by the initial neutral cluster temperature ( T ≈ 100 K) and the energy transfer in the ionizing collision. In addition, the comparison between the measured and simulated spectra suggests for high cluster charges a multi-fragmentation process, in which most of charge is emitted, creating low charged residual cluster ions. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index