Assembled Porphyrin Nanofiber on the Surface of g-C 3 N 4 Nanomaterials for Enhanced Photocatalytic Degradation of Organic Dyes.

Autor: Lai, Hoan Thi, Nguyen, Giang Thi, Tran, Nga Thuy, Nguyen, Thanh Tung, Van Tran, Chinh, Nguyen, Duy Khiem, Chang, S. W., Chung, W. Jin, Nguyen, Dinh Duc, Thi, Hoai Phuong Nguyen, La, Duong Duc
Předmět:
Zdroj: Catalysts (2073-4344); Dec2022, Vol. 12 Issue 12, p1630, 13p
Abstrakt: In this work, a g-C3N4/porphyrin nanocomposite was fabricated through the self-assembling of monomeric Tetrakis (4-carboxyphenyl) porphyrin (TCPP) molecules with g-C3N4 nanomaterials. The characterizing results showed a good distribution of TCPP nanofibers with a diameter of < 100 nm and several micrometers in length on the g-C3N4 nanoflakes' surfaces. The prepared g-C3N4/porphyrin nanocomposite had two bandgap energies of 2.38 and 2.7 eV, which could harvest a wide range of photon energy in the light spectrum, particularly in visible light. The obtained C3N4/TCPP nanocomposite revealed a remarkable photodegradation efficiency toward rhodamine B dyes, with a RhB removing rate of 3.3 × 10−2 min−1. The plausible mechanism for the photocatalytic performance of the g-C3N4/porphyrin photocatalyst for the RhB dye's degradation was also studied and discussed. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index
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