Tantalum Suboxide Films with Tunable Composition and Electrical Resistivity Deposited by Reactive Magnetron Sputtering.

Autor: Baker, Alexander A., Engwall, Alison M., Bayu-Aji, Leonardus Bimo, Bae, John H., Shin, Swanee J., Moody, John D., Kucheyev, Sergei O.
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Zdroj: Coatings (2079-6412); Jul2022, Vol. 12 Issue 7, pN.PAG-N.PAG, 10p
Abstrakt: Tantalum-based films with tailored composition, density, and electrical resistivity are of interest for next generation hohlraums for magnetized indirect-drive inertial confinement fusion. Here, we use reactive direct-current magnetron sputtering to deposit tantalum suboxide films with O content in the range of 46–71 at.%. In contrast to a common approach involving varying reactive gas contents, compositional control is achieved kinetically by changing the total chamber pressure and the deposition rate, while keeping the working gas mix of Ar-5%O 2 constant. The resultant films are X-ray amorphous with electrical resistivity varying by over seven orders of magnitude. The dominant conduction mechanism changes from metallic to activated tunneling above ∼55 at.% of O, which is characterized by a sharp increase in resistivity and a decrease in the carrier density at low temperatures. [ABSTRACT FROM AUTHOR]
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