High harmonic generation in two-dimensional Mott insulators.

Autor: Orthodoxou, Christopher, Zaïr, Amelle, Booth, George H.
Předmět:
Zdroj: NPJ Quantum Materials; 9/9/2021, Vol. 6 Issue 1, p1-8, 8p
Abstrakt: With a combination of numerical methods, including quantum Monte Carlo, exact diagonalization, and a simplified dynamical mean-field model, we consider the attosecond charge dynamics of electrons induced by strong-field laser pulses in two-dimensional Mott insulators. The necessity to go beyond single-particle approaches in these strongly correlated systems has made the simulation of two-dimensional extended materials challenging, and we contrast their resulting high-harmonic emission with more widely studied one-dimensional analogues. As well as considering the photo-induced breakdown of the Mott insulating state and magnetic order, we also resolve the time and ultra-high-frequency domains of emission, which are used to characterize both the photo-transition, and the sub-cycle structure of the electron dynamics. This extends simulation capabilities and understanding of the photo-melting of these Mott insulators in two dimensions, at the frontier of attosecond non-equilibrium science of correlated materials. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index