Fractional revivals in the rovibrational motion of I2.

Autor: Lohmuller, T., Engel, V., Beswick, J. A., Meier, C.
Předmět:
Zdroj: Journal of Chemical Physics; 6/8/2004, Vol. 120 Issue 22, p10442-10449, 8p, 4 Graphs
Abstrakt: Motivated by pump—probe experiments of I2 in a room-temperature sample, the detection of fractional revivals is investigated using full-dimensional quantum wave packet calculations. It is shown that the structures observed in the pump—probe signal depend sensitively on the probe parameters employed and that the observed signal reflects a particular phase effect between fractional revivals. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index