Multiple core-hole formation by free-electron laser radiation in molecular nitrogen.

Autor: H I B Banks, D A Little, A Emmanouilidou
Předmět:
Zdroj: Journal of Physics B: Atomic, Molecular & Optical Physics; 5/14/2018, Vol. 51 Issue 9, p1-1, 1p
Abstrakt: We investigate the formation of multiple-core-hole states of molecular nitrogen interacting with a free-electron laser pulse. In previous work, we obtained bound and continuum molecular orbitals in the single-center expansion scheme and used these orbitals to calculate photo-ionization and auger decay rates. We extend our formulation to track the proportion of the population that accesses single-site versus two-site double-core-hole (TSDCH) states, before the formation of the final atomic ions. We investigate the pulse parameters that favor the formation of the single-site and TSDCH as well as triple-core-hole states for 525 and 1100 eV photons. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index