Pump−probe experiments at the TEMPO beamline using the low-α operation mode of Synchrotron SOLEIL.

Autor: Silly, Mathieu G., Ferté, Tom, Tordeux, Marie Agnes, Pierucci, Debora, Beaulieu, Nathan, Chauvet, Christian, Pressacco, Federico, Sirotti, Fausto, Popescu, Horia, Lopez-Flores, Victor, Tortarolo, Marina, Sacchi, Maurizio, Jaouen, Nicolas, Hollander, Philippe, Ricaud, Jean Paul, Bergeard, Nicolas, Boeglin, Christine, Tudu, Bharati, Delaunay, Renaud, Luning, Jan
Předmět:
Zdroj: Journal of Synchrotron Radiation; Jul2017, Vol. 24 Issue 4, p886-897, 11p
Abstrakt: The SOLEIL synchrotron radiation source is regularly operated in special filling modes dedicated to pump-probe experiments. Among others, the low-α mode operation is characterized by shorter pulse duration and represents the natural bridge between 50 ps synchrotron pulses and femtosecond experiments. Here, the capabilities in low-α mode of the experimental set-ups developed at the TEMPO beamline to perform pump-probe experiments with soft X-rays based on photoelectron or photon detection are presented. A 282 kHz repetition-rate femtosecond laser is synchronized with the synchrotron radiation time structure to induce fast electronic and/or magnetic excitations. Detection is performed using a two-dimensional space resolution plus time resolution detector based on microchannel plates equipped with a delay line. Results of time-resolved photoelectron spectroscopy, circular dichroism and magnetic scattering experiments are reported, and their respective advantages and limitations in the framework of high-time-resolution pump-probe experiments compared and discussed. [ABSTRACT FROM AUTHOR]
Databáze: Complementary Index