Flexible X-Ray Detector for Cumulative Dose Monitoring Through Reversible Photochromism and Luminescence Modulation.

Autor: Bai X; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China., Zhang Y; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China., Zhao H; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China.; Southwest United Graduate School, Kunming, 650092, China., Zi Y; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China.; Southwest United Graduate School, Kunming, 650092, China., Xu Z; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China., Huang A; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China., Cun Y; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China., Liu Y; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China., Song Z; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China., Qiu J; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China., Liao J; Institute for Biomedical Materials and Devices (IBMD), Faculty of Science, University of Technology Sydney, Sydney, NSW, 2007, Australia., Yang Z; College of Materials Science and Engineering, Kunming University of Science and Technology, Kunming, 650093, China.; Southwest United Graduate School, Kunming, 650092, China.
Jazyk: angličtina
Zdroj: Advanced science (Weinheim, Baden-Wurttemberg, Germany) [Adv Sci (Weinh)] 2024 Dec 23, pp. e2412986. Date of Electronic Publication: 2024 Dec 23.
DOI: 10.1002/advs.202412986
Abstrakt: This study presents a multi-mode X-ray detection and imaging strategy by integrating photochromism, photoluminescence, and radioluminescence into Tb 3+ -doped CaAl 2 Si 2 O 8 . CaAl 2 Si 2 O 8 : Tb 3+ exhibits stable radioluminescence, oxygen vacancy-related photochromism, and photoluminescence modulation, all of which showed a linear relationship with X-ray exposure. This multi-mode response enables high-quality imaging and detection in both bright and dark conditions, facilitating time-dependent cumulative X-ray radiation dose assessments. Reversible color and luminescence changes are achieved through cyclic tests involving alternating X-ray and 473 nm laser irradiation. The PDMS CaAl 2 Si 2 O 8 : Tb 3+ ink and flexible film demonstrate high suitability for wearable X-ray detection devices and imaging of irregular objects, offering an innovative approach to X-ray detection and imaging.
(© 2024 The Author(s). Advanced Science published by Wiley‐VCH GmbH.)
Databáze: MEDLINE