Syngas enhancement for Fischer-Tropsch integration via solid oxide electrolyzer cell co-electrolysis with or without methane.

Autor: Machado M; Instituto SENAI de Inovação em Biomassa - ISI Biomassa, SENAI-MS, Av Angelina Tebet, 777, Três Lagoas 79640-250, MS, Brazil., de Souza Junior RL; Instituto de Química, Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 21941-909, RJ, Brazil.; LIPCAT (Laboratório de Intensificação de Processos e Catálise), Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 21941-594, RJ, Brazil., de Almeida JMAR; Instituto de Química, Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 21941-909, RJ, Brazil.; LIPCAT (Laboratório de Intensificação de Processos e Catálise), Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 21941-594, RJ, Brazil., Romano PN; LIPCAT (Laboratório de Intensificação de Processos e Catálise), Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 21941-594, RJ, Brazil.; Campus Duque de Caxias, Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 25245-390, Brazil.; Nanotechnology Engineering Program, Alberto Luiz Coimbra Institute for Graduate Studies and Research in Engineering, COPPE, Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 21941-972, RJ, Brazil., Garcia MAS; LIPCAT (Laboratório de Intensificação de Processos e Catálise), Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 21941-594, RJ, Brazil.; Nanotechnology Engineering Program, Alberto Luiz Coimbra Institute for Graduate Studies and Research in Engineering, COPPE, Universidade Federal do Rio de Janeiro (UFRJ), Rio de Janeiro 21941-972, RJ, Brazil.; Department of Chemistry, Federal University of Maranhão (UFMA), São Luís 65080-805, MA, Brazil.
Jazyk: angličtina
Zdroj: IScience [iScience] 2024 Sep 23; Vol. 27 (10), pp. 111014. Date of Electronic Publication: 2024 Sep 23 (Print Publication: 2024).
DOI: 10.1016/j.isci.2024.111014
Abstrakt: The transition toward a sustainable energy framework requires developing innovative methods for fuel generation that utilize renewable resources and decrease carbon footprints. Thus, the review overviews current advancements in solid oxide electrolysis cell (SOEC) technology, specifically focusing on its application in co-electrolysis processes to produce syngas with different H 2 :CO ratios, essential for Fischer-Tropsch synthesis. It emphasizes the potential of integrating partial methane oxidation reaction into the electrolysis process. By examining recent developments in electrode, electrolyte materials, and system design, the review highlights how these technological enhancements can reduce energy consumption, improve system durability, and facilitate the integration of renewable energy sources. Additionally, the role of methane assistance in SOECs is discussed, illustrating its impact on operational efficiency. Then, future research directions that could optimize syngas production and expand the applicability of SOEC technology in industrial settings are proposed, supporting the transition to a more sustainable energy landscape.
Competing Interests: There are no conflicts of interest to disclose.
(© 2024 The Author(s).)
Databáze: MEDLINE
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