Development of a Photothermal Regenerative Plasmonic Platform as a Light-Controlled Interface.

Autor: Guglielmelli A; Nanoscience Laboratory for Human Technologies (NLHT) Lab, Department of Physics, Institute of Nanotechnology (CNR-Nanotec), University of Calabria, 87036 Rende, Italy., Mazzei R; Institute on Membrane Technology (ITM-CNR), National Research Council, 87036 Rende, Italy., Palermo G; Nanoscience Laboratory for Human Technologies (NLHT) Lab, Department of Physics, Institute of Nanotechnology (CNR-Nanotec), University of Calabria, 87036 Rende, Italy., Valente L; NLHT Lab, Department of Physics, University of Calabria, 87036 Rende, Italy., Tone CM; Department of Physics, Molecular Physics Group, University of Calabria, 87036 Rende, Italy., Giorno L; Institute on Membrane Technology (ITM-CNR), National Research Council, 87036 Rende, Italy., Strangi G; Nanoscience Laboratory for Human Technologies (NLHT) Lab, Department of Physics, Institute of Nanotechnology (CNR-Nanotec), University of Calabria, 87036 Rende, Italy.; Department of Physics, Case Western Reserve University, Cleveland, Ohio 44106, United States., Poerio T; Institute on Membrane Technology (ITM-CNR), National Research Council, 87036 Rende, Italy.
Jazyk: angličtina
Zdroj: ACS applied materials & interfaces [ACS Appl Mater Interfaces] 2024 Oct 30; Vol. 16 (43), pp. 59586-59596. Date of Electronic Publication: 2024 Oct 18.
DOI: 10.1021/acsami.4c13455
Abstrakt: This study introduces a novel plasmonic nanocomposite platform, where gold nanoparticles (AuNPs) are synthesized in situ within a polydimethylsiloxane (PDMS) film. The innovative fabrication process leverages ethyl acetate swelling to achieve a uniform distribution of AuNPs, eliminating the need for additional reagents. The resulting nanocomposite film exhibits exceptional photothermal conversion capabilities, efficiently converting absorbed light into heat and rapidly reaching high temperatures. Furthermore, the platform is biofunctionalized with the phosphotriesterase enzyme, not only enabling the degradation of organophosphate pesticides but also showcasing the potential for multifunctional applications. The platform's ability to be regenerated after use underscores its sustainability for repeated applications.
Databáze: MEDLINE