Stability and degradation of (oxy)nitride photocatalysts for solar water splitting.

Autor: Werner V; Department of Chemistry and Physics of Materials, Paris Lodron University Salzburg Jakob-Haringer-Str. 2A 5020 Salzburg Austria simone.pokrant@plus.ac.at., Lora FB; Laboratory of Renewable Energy Science and Engineering, Ecole Polytechnique Fédérale de Lausanne 1015 Lausanne Switzerland., Chai Z; Department of Chemistry, University of Zurich Winterthurerstrasse 190 CH-8057 Zurich Switzerland., Hörndl J; Department of Chemistry and Physics of Materials, Paris Lodron University Salzburg Jakob-Haringer-Str. 2A 5020 Salzburg Austria simone.pokrant@plus.ac.at., Praxmair J; Department of Chemistry and Physics of Materials, Paris Lodron University Salzburg Jakob-Haringer-Str. 2A 5020 Salzburg Austria simone.pokrant@plus.ac.at., Luber S; Department of Chemistry, University of Zurich Winterthurerstrasse 190 CH-8057 Zurich Switzerland., Haussener S; Laboratory of Renewable Energy Science and Engineering, Ecole Polytechnique Fédérale de Lausanne 1015 Lausanne Switzerland., Pokrant S; Department of Chemistry and Physics of Materials, Paris Lodron University Salzburg Jakob-Haringer-Str. 2A 5020 Salzburg Austria simone.pokrant@plus.ac.at.
Jazyk: angličtina
Zdroj: RSC sustainability [RSC Sustain] 2024 May 02; Vol. 2 (6), pp. 1738-1752. Date of Electronic Publication: 2024 May 02 (Print Publication: 2024).
DOI: 10.1039/d4su00096j
Abstrakt: Advancing towards alternative technologies for the sustainable production of hydrogen is a necessity for the successful integration of this potentially green fuel in the future. Photocatalytic and photoelectrochemical water splitting are promising concepts in this context. Over the past decades, researchers have successfully explored several materials classes, such as oxides, nitrides, and oxynitrides, in their quest for suitable photocatalysts with a focus on reaching higher efficiencies. However, to pave the way towards practicability, understanding degradation processes and reaching stability is essential, a domain where research has been scarcer. This perspective aims at providing an overview on recent progress concerning stability and degradation with a focus on (oxy)nitride photocatalysts and at providing insights into the opportunities and challenges coming along with the investigation of degradation processes and the attempts to improve the stability of photocatalysts.
Competing Interests: There are no conflicts to declare.
(This journal is © The Royal Society of Chemistry.)
Databáze: MEDLINE