Engineering the Impact of Phonon Dephasing on the Coherence of a WSe_{2} Single-Photon Source via Cavity Quantum Electrodynamics.

Autor: Mitryakhin VN; Carl von Ossietzky Universität Oldenburg, Fakultät V, Institut für Physik, 26129 Oldenburg, Germany., Steinhoff A; Institute for Theoretical Physics and Bremen Center for Computational Material Science, University of Bremen, 28334 Bremen, Germany., Drawer JC; Carl von Ossietzky Universität Oldenburg, Fakultät V, Institut für Physik, 26129 Oldenburg, Germany., Shan H; Carl von Ossietzky Universität Oldenburg, Fakultät V, Institut für Physik, 26129 Oldenburg, Germany., Florian M; University of Michigan, Department of Electrical Engineering and Computer Science, Ann Arbor, Michigan 48109, USA., Lackner L; Carl von Ossietzky Universität Oldenburg, Fakultät V, Institut für Physik, 26129 Oldenburg, Germany., Han B; Carl von Ossietzky Universität Oldenburg, Fakultät V, Institut für Physik, 26129 Oldenburg, Germany., Eilenberger F; Friedrich Schiller University Jena, Jena, Germany., Tongay SA; Materials Science and Engineering, School for Engineering of Matter, Transport and Energy, Arizona State University, Tempe, Arizona 85287, USA., Watanabe K; Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan., Taniguchi T; International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan., Antón-Solanas C; Depto. de Física de Materiales, Instituto Nicolás Cabrera, Instituto de Física de la Materia Condensada, Universidad Autónoma de Madrid, 28049 Madrid, Spain., Predojević A; Carl von Ossietzky Universität Oldenburg, Fakultät V, Institut für Physik, 26129 Oldenburg, Germany.; Department of Physics, Stockholm University, 10691 Stockholm, Sweden., Gies C; Institute for Theoretical Physics and Bremen Center for Computational Material Science, University of Bremen, 28334 Bremen, Germany., Esmann M; Carl von Ossietzky Universität Oldenburg, Fakultät V, Institut für Physik, 26129 Oldenburg, Germany., Schneider C; Carl von Ossietzky Universität Oldenburg, Fakultät V, Institut für Physik, 26129 Oldenburg, Germany.
Jazyk: angličtina
Zdroj: Physical review letters [Phys Rev Lett] 2024 May 17; Vol. 132 (20), pp. 206903.
DOI: 10.1103/PhysRevLett.132.206903
Abstrakt: Emitter dephasing is one of the key issues in the performance of solid-state single-photon sources. Among the various sources of dephasing, acoustic phonons play a central role in adding decoherence to the single-photon emission. Here, we demonstrate that it is possible to tune and engineer the coherence of photons emitted from a single WSe_{2} monolayer quantum dot via selectively coupling it to a spectral cavity resonance. We utilize an open cavity to demonstrate spectral enhancement, leveling, and suppression of the highly asymmetric phonon sideband, finding excellent agreement with a microscopic description of the exciton-phonon dephasing in a truly two-dimensional system. Moreover, the impact of cavity tuning on the dephasing is directly assessed via optical interferometry, which points out the capability to utilize light-matter coupling to steer and design dephasing and coherence of quantum emitters in atomically thin crystals.
Databáze: MEDLINE