Engineering Electronic Structure of Nitrogen-Carbon Sites by sp 3 -Hybridized Carbon and Incorporating Chlorine to Boost Oxygen Reduction Activity.
Autor: | Feng X; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China., Chen G; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China., Cui Z; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China., Qin R; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China., Jiao W; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China., Huang Z; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China., Shang Z; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China., Ma C; Department of Chemistry, Tsinghua University, Beijing, 100084, China., Zheng X; National Synchrotron Radiation Laboratory University of Science and Technology of China, Hefei, Anhui, 230029, China., Han Y; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China., Huang W; Institute of Flexible Electronics (IFE), Ningbo Institute, and Frontiers Science Center for Flexible Electronics, Northwestern Polytechnical University, Xi'an, 710072, China. |
---|---|
Jazyk: | angličtina |
Zdroj: | Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2024 Jan 02; Vol. 63 (1), pp. e202316314. Date of Electronic Publication: 2023 Nov 30. |
DOI: | 10.1002/anie.202316314 |
Abstrakt: | Development of efficient and easy-to-prepare low-cost oxygen reaction electrocatalysts is essential for widespread application of rechargeable Zn-air batteries (ZABs). Herein, we mixed NaCl and ZIF-8 by simple physical milling and pyrolysis to obtain a metal-free porous electrocatalyst doped with Cl (mf-pClNC). The mf-pClNC electrocatalyst exhibits a good oxygen reduction reaction (ORR) activity (E (© 2023 Wiley-VCH GmbH.) |
Databáze: | MEDLINE |
Externí odkaz: |