The seasonal change of PAHs in Svalbard surface snow.
Autor: | Vecchiato M; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy. Electronic address: vecchiato@unive.it., Barbante C; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Barbaro E; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Burgay F; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Laboratory of Environmental Chemistry (LUC), Paul Scherrer Institut (PSI), 5232, Villigen, Switzerland., Cairns WR; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Callegaro A; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Cappelletti D; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Department of Chemistry, Biology and Biotechnology, University of Perugia, 06123, Perugia, Italy., Dallo F; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., D'Amico M; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Feltracco M; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Gallet JC; Norwegian Polar Institute, 9296, Tromsø, Norway., Gambaro A; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Larose C; Univ Lyon, CNRS, INSA Lyon, Université Claude Bernard Lyon 1, Ecole Centrale de Lyon, Ampère, UMR5005, 69134, Ecully, Cedex, France., Maffezzoli N; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Mazzola M; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Sartorato I; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Scoto F; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Atmospheric Sciences and Climate - National Research Council (ISAC-CNR), Campus Ecotekne, 73100, Lecce, Italy., Turetta C; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Vardè M; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy., Xie Z; Institute of Coastal Environmental Chemistry, Helmholtz-Zentrum Hereon, 21502, Geesthacht, Germany., Spolaor A; Department of Environmental Sciences, Informatics and Statistics (DAIS), Ca' Foscari University of Venice, Via Torino 155, 30172, Venezia-Mestre, Venice, Italy; Institute of Polar Sciences - National Research Council (ISP-CNR), Via Torino 155, 30172, Venezia-Mestre, Venice, Italy. |
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Jazyk: | angličtina |
Zdroj: | Environmental pollution (Barking, Essex : 1987) [Environ Pollut] 2024 Jan 01; Vol. 340 (Pt 1), pp. 122864. Date of Electronic Publication: 2023 Nov 02. |
DOI: | 10.1016/j.envpol.2023.122864 |
Abstrakt: | The Arctic region is threatened by contamination deriving from both long-range pollution and local human activities. Polycyclic Aromatic Hydrocarbons (PAHs) are environmental tracers of emission, transport and deposition processes. A first campaign has been conducted at Ny-Ålesund, Svalbard, from October 2018 to May 2019, monitoring weekly concentrations of PAHs in Arctic surface snow. The trend of the 16 high priority PAH compounds showed that long-range inputs occurred mainly in the winter, with concentrations ranging from 0.8 ng L -1 to 37 ng L -1 . In contrast to this, the most abundant analyte retene, showed an opposite seasonal trend with highest values in autumn and late spring (up to 97 ng L -1 ), while in winter this compound remained below 3 ng L -1 . This is most likely due to local contributions from outcropping coal deposits and stockpiles. Our results show a general agreement with the atmospheric signal, although significant skews can be attributed to post-depositional processes, wind erosion, melting episodes and redistribution. Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper. (Copyright © 2023 The Authors. Published by Elsevier Ltd.. All rights reserved.) |
Databáze: | MEDLINE |
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