Exploring the capture and desorption of CO 2 on graphene oxide foams supported by computational calculations.

Autor: Arango Hoyos BE; Energy Engineering, Faculty of Engineering and Sciences, Universidad Adolfo Ibáñez, 7941169, Santiago, Chile., Osorio HF; Electronic Instrumentation Technology Program, Faculty of Basic Science and Technology, Universidad del Quindío, 630001, Armenia, Colombia., Valencia Gómez EK; Doctoral Program in Physical Sciences, Interdisciplinary Institute of Sciences, Universidad del Quindío, 630004, Armenia, Colombia., Guerrero Sánchez J; Virtual Materials Modeling Laboratory (LVMM), Center for Nanoscience and Nanotechnology, Universidad Nacional Autónoma de México, Ensenada, 22860, Mexico., Del Canto Palominos AP; Energy Engineering, Faculty of Engineering and Sciences, Universidad Adolfo Ibáñez, 7941169, Santiago, Chile., Larrain FA; Energy Engineering, Faculty of Engineering and Sciences, Universidad Adolfo Ibáñez, 7941169, Santiago, Chile., Prías Barragán JJ; Electronic Instrumentation Technology Program, Faculty of Basic Science and Technology, Universidad del Quindío, 630001, Armenia, Colombia. jjprias@uniquindio.edu.co.; Doctoral Program in Physical Sciences, Interdisciplinary Institute of Sciences, Universidad del Quindío, 630004, Armenia, Colombia. jjprias@uniquindio.edu.co.
Jazyk: angličtina
Zdroj: Scientific reports [Sci Rep] 2023 Sep 02; Vol. 13 (1), pp. 14476. Date of Electronic Publication: 2023 Sep 02.
DOI: 10.1038/s41598-023-41683-4
Abstrakt: In the last decade, the highest levels of greenhouse gases (GHG) in the atmosphere have been recorded, with carbon dioxide (CO 2 ) being one of the GHGs that most concerns mankind due to the rate at which it is generated on the planet. Given its long time of permanence in the atmosphere (between 100 to 150 years); this has deployed research in the scientific field focused on the absorption and desorption of CO 2 in the atmosphere. This work presents the study of CO 2 adsorption employing materials based on graphene oxide (GO), such as GO foams with different oxidation percentages (3.00%, 5.25%, and 9.00%) in their structure, obtained via an environmentally friendly method. The characterization of CO 2 adsorption was carried out in a closed system, within which were placed the GO foams and other CO 2 adsorbent materials (zeolite and silica gel). Through a controlled chemical reaction, production of CO 2 was conducted to obtain CO 2 concentration curves inside the system and calculate from these the efficiency, obtained between 86.28 and 92.20%, yield between 60.10 and 99.50%, and effectiveness of CO 2 adsorption of the materials under study. The results obtained suggest that GO foams are a promising material for carbon capture and the future development of a new clean technology, given their highest CO 2 adsorption efficiency and yield.
(© 2023. Springer Nature Limited.)
Databáze: MEDLINE
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