Intrinsically Stretchable Organic Electrochemical Transistors with Rigid-Device-Benchmarkable Performance.

Autor: Liu D; Department of Electrical and Electronic Engineering, The University of Hong Kong, Hong Kong SAR, China., Tian X; Department of Electrical and Electronic Engineering, The University of Hong Kong, Hong Kong SAR, China., Bai J; Department of Electrical and Electronic Engineering, The University of Hong Kong, Hong Kong SAR, China., Wang Y; Department of Electrical and Electronic Engineering, The University of Hong Kong, Hong Kong SAR, China., Cheng Y; Department of Electrical and Electronic Engineering, The University of Hong Kong, Hong Kong SAR, China., Ning W; Department of Electrical and Electronic Engineering, The University of Hong Kong, Hong Kong SAR, China., Chan PKL; Department of Mechanical Engineering, The University of Hong Kong, Hong Kong SAR, China., Wu K; State Key Laboratory of Polymer Materials Engineering, College of Polymer Science and Engineering, Sichuan University, Chengdu, 610065, China., Sun J; State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, 130012, China., Zhang S; Department of Electrical and Electronic Engineering, The University of Hong Kong, Hong Kong SAR, China.
Jazyk: angličtina
Zdroj: Advanced science (Weinheim, Baden-Wurttemberg, Germany) [Adv Sci (Weinh)] 2022 Oct; Vol. 9 (29), pp. e2203418. Date of Electronic Publication: 2022 Jul 29.
DOI: 10.1002/advs.202203418
Abstrakt: Intrinsically stretchable organic electrochemical transistors (OECTs) are being pursued as the next-generation tissue-like bioelectronic technologies to improve the interfacing with the soft human body. However, the performance of current intrinsically stretchable OECTs is far inferior to their rigid counterparts. In this work, for the first time, the authors report intrinsically stretchable OECTs with overall performance benchmarkable to conventional rigid devices. In particular, oxygen level in the stretchable substrate is revealed to have a significant impact on the on/off ratio. By employing stretchable substrates with low oxygen permeabilities, the on/off ratio is elevated from ≈10 to a record-high value of ≈10 4 , which is on par with a rigid OECT. The device remained functional after cyclic stretching tests. This work demonstrates that intrinsically stretchable OECTs have the potential to serve as a new building block for emerging soft bioelectronic applications such as electronic skin, soft implantables, and soft neuromorphic computing.
(© 2022 The Authors. Advanced Science published by Wiley-VCH GmbH.)
Databáze: MEDLINE
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