Occurrence, concentration, and distribution of 38 organic micropollutants in the filter material of 12 stormwater bioretention facilities.

Autor: Furén R; Urban Water Engineering, Department of Civil, Environmental and Natural Resources Engineering, Luleå University of Technology, 971 87 Luleå, Sweden; NCC Sverige AB, Department of Research & Innovation, 170 80 Solna, Sweden. Electronic address: rober.furen@associated.ltu.se., Flanagan K; Urban Water Engineering, Department of Civil, Environmental and Natural Resources Engineering, Luleå University of Technology, 971 87 Luleå, Sweden., Winston RJ; Department of Food, Agricultural, and Biological Engineering, The Ohio State University, Columbus, OH, United States; Department of Civil, Environmental, and Geodetic Engineering, The Ohio State University, Columbus, OH, United States., Tirpak RA; Department of Food, Agricultural, and Biological Engineering, The Ohio State University, Columbus, OH, United States., Dorsey JD; Department of Food, Agricultural, and Biological Engineering, The Ohio State University, Columbus, OH, United States., Viklander M; Urban Water Engineering, Department of Civil, Environmental and Natural Resources Engineering, Luleå University of Technology, 971 87 Luleå, Sweden., Blecken GT; Urban Water Engineering, Department of Civil, Environmental and Natural Resources Engineering, Luleå University of Technology, 971 87 Luleå, Sweden.
Jazyk: angličtina
Zdroj: The Science of the total environment [Sci Total Environ] 2022 Nov 10; Vol. 846, pp. 157372. Date of Electronic Publication: 2022 Jul 16.
DOI: 10.1016/j.scitotenv.2022.157372
Abstrakt: The increased use of bioretention facilities as a low impact development measure for treating stormwater runoff underscores the need to further understand their long-term function. Eventually, bioretention filter media must be (partly) replaced and disposed of at the end of its functional lifespan. While there are several studies of metal accumulation and distributions in bioretention media, less is known about organic pollutant pathways and accumulation in these filters. The present study considers the occurrence and accumulation of 16 polycyclic aromatic hydrocarbons, 7 polychlorinated biphenyls, 13 phthalates, and two alkylphenols throughout 12 older bioretention facilities (7-13 years old) used for stormwater treatment in Michigan and Ohio, USA. These pollutant groups appear to behave similarly, with greater instances of detection and higher concentrations in the upper media layers which decrease with increased depth from the surface. The patterns of detection and concentration in the filter material may be explained by characteristics of the pollutants, such as molecular structures and solubility that affect the removal of the organic pollutants by the filter material. There is also a large variation in concentration magnitudes between the bioretention sites, most likely due to differences in pollutant sources, contributing catchment size and/or land uses.
Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
(Copyright © 2022. Published by Elsevier B.V.)
Databáze: MEDLINE