Defect-induced ultimately fast volume phonon-polaritons in the wurtzite Zn 0.74 Mg 0.26 Se mixed crystal.

Autor: Dicko H; LCP-A2MC, Institut Jean Barriol, Université de Lorraine, Metz, F-57078, France., Pagès O; LCP-A2MC, Institut Jean Barriol, Université de Lorraine, Metz, F-57078, France. olivier.pages@univ-lorraine.fr., Shoker MB; LCP-A2MC, Institut Jean Barriol, Université de Lorraine, Metz, F-57078, France., Firszt F; Institute of Physics, N. Copernicus University, 87-100, Toruń, Poland., Strzałkowski K; Institute of Physics, N. Copernicus University, 87-100, Toruń, Poland., Maillard A; LMOPS, Université de Lorraine - Supélec, 2 rue Edouard Belin, F-57070, Metz, France., Polian A; Institut de Minéralogie, de Physique des Matériaux et de Cosmochimie, Sorbonne Université -UMR CNRS 7590, F-75005, Paris, France., Battie Y; LCP-A2MC, Institut Jean Barriol, Université de Lorraine, Metz, F-57078, France., Broch L; LCP-A2MC, Institut Jean Barriol, Université de Lorraine, Metz, F-57078, France., En Naciri A; LCP-A2MC, Institut Jean Barriol, Université de Lorraine, Metz, F-57078, France., Postnikov AV; LCP-A2MC, Institut Jean Barriol, Université de Lorraine, Metz, F-57078, France., Paszkowicz W; Institute of Physics, Polish Academy of Sciences, Aleja Lotników 32/46, PL-02668, Warsaw, Poland., Itié JP; Synchrotron SOLEIL, L'Orme des Merisiers Saint-Aubin, BP 48, F-91192, Gif-sur-Yvette Cedex, France.
Jazyk: angličtina
Zdroj: Scientific reports [Sci Rep] 2019 May 24; Vol. 9 (1), pp. 7817. Date of Electronic Publication: 2019 May 24.
DOI: 10.1038/s41598-019-44273-5
Abstrakt: Volume-phonon-polaritons (VPP's) propagating at a light-in-vacuum-like speed are identified in the wurtzite-type Zn 0.74 Mg 0.26 Se mixed crystal by near-forward Raman scattering. Their detection is selective to both the laser energy and the laser polarization, depending on whether the ordinary (n 0 ) or extraordinary (n e ) refractive index is addressed. Yet, no significant linear birefringence (n 0  [Formula: see text] n e ) is observed by ellipsometry. The current access to ultrafast VPP's is attributed to the quasi-resonant Raman probing of an anomalous dispersion of n 0 due to impurity levels created deep in the optical band gap by oriented structural defects. The resonance conditions are evidenced by a dramatic enhancement of the Raman signals due to the polar modes. Hence, this work reveals a capacity for the lattice defects' engineering to "accelerate" the VPP's of a mixed crystal up to light-in-vacuum-like speeds. This is attractive for ultrafast signal processing in the terahertz range. On the fundamental side we provide an insight into the VPP's created by alloying ultimately close to the center of the Brillouin zone.
Databáze: MEDLINE
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